Well he's pure evil no doubt. But I would have had Dimentio or Sidous as "just evil". But tragic villains are my favorite. Lotso, Count Bleck, Killing Joke, Telltale and 2019 Joker etc.
I personally think that redeemed villains are the best. You get to see their journey from a villain to becoming a better person. Also, a lot of redeemed villains also have interesting backstories and reasons to redeem themselves, making it 2 in one.