I really want him to analyze Gendo Ikari from Evangelion, Kilgrave from Jessica Jones, and Prince Lotor from Voltron.

The Ink Demon

I'd like to see Albert Wesker, Vladimir Makarov and Grant Ward covered

Catra and Horde Prime from She-Ra

Some villains from Starcraft or Warcraft (though, I am pretty sure he is never going to analyze characters from these, unfortunately)

Sauron

Alan Yates (i have been asking for an Alan Yates episode for months now IT WILL HAPPEN)