Villains in Japanese animation with expressive features and symbolism not always found in other forms of animation. Anime characters are depicted with traits more realistic and/or less cartoonish, especially when compared to Western media. This often overlaps with Manga Villains due to manga being adapted into anime and vice versa.
IMPORTANT: Do NOT add Villains from Western animation, as they belong in Cartoon Villains, regardless of whether or not they were anime-inspired or anime-esque, though they might be considered characters from anime imitations (i.e. The Boondocks, Avatar: The Last Airbender, The Legend of Korra, RWBY).
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- A-Laws
- Aaroniero Arruruerie
- Abel (Fairy Tail)
- Abel (Saint Seiya)
- Aber Rindt
- Abidos the Third
- Abil
- Abirama Redder
- Abnes
- Abo
- Abrego
- Absalom
- Abyss Trinity
- Abyssal Fleet
- Abzu
- Acceleration Research Society
- Accelerator
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- Achilles (Cyborg 009)
- Achilles (Mazinger)
- Acidwire
- Acnologia
- Acqua of the Back
- Acro
- Adam (Black Cat)
- Adam Arclight
- Adam Weishaupt
- Adamski
- Adiane the Elegant
- Admiral Haruki Kusakabe
- Admiral Perry
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- Adolf Hitler (Drifters)
- Adolf Hitler (Fullmetal Alchemist)
- Adon Coborlwitz
- ADR-01: Jeri Type
- Aegaeon
- Aegir
- Aether Foundation
- Afro Droid
- Agata
- Agnese Forces
- Agnese Sanctis
- Ahbmad Saluja
- Ai Imari
- Ai Magase
- Aiguille Delaz
- Aileen Rao
- Ain
- Aina Sahalin
- Aine
- Ainz Ooal Gown
- Aircraft Carrier Princess
- Airfield Princess
- Airi
- AirMan.EXE
- Airzel
- Aisrehdar
- Aisslinger Wernarr
- Ajeel Ramal
- Ak-Baba
- Aka
- Akahoshi
- Akai
- Akainu
- Akakabuto
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- Akane Hiyama
- Akasha Shishidou (Corpse Princess)
- Akatsuki
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- Akatsuki (Ojamajo Doremi)
- Akaza
- Akechi Mitsuhide
- Akemi Hinazuki
- Aki Honda
- Aki Myojin
- Aki Tsukino
- Akihiko Kayaba
- Akihiro Kanou
- Akihiro Kurata
- Akio Ohtori
- Akira Otoishi
- Akira Takaoka
- Akito Hyuga
- Akito Sohma
- Akito Sohma (Fruits Basket 2001)
- Akudaikan
- Akuma
- Akuma Shogun
- Akura-Ou
- Akutagawa Ryuunosuke
- Akācho
- Al-Thamen
- Alakazam
- Alala
- Alan and Ann
- Alan Sylvasta
- Alaskan Base Offficer
- Alastor
- Alauda Hafez
- Alba
- Albedo (Overlord)
- Albedo Piazzolla
- Alberich XIII
- Albert de Blois
- Albert Maverick
- Albertine
- Aldegor
- Aldith
- Aldra
- Aleistor Chamber
- Alejandro Corner
- Alekteus
- Alessi
- Alex & Mueller
- Alex Rosewater
- Alexander Anderson
- Alexander Anderson (Team Four Star)
- Alexei Barnes Alderp
- Alexei Dionia
- Alexis Leskinen
- Alexis • Kerib
- Alfred, Duke of Meinz
- Ali Al-Saachez
- Aliana
- Alice Miller
- Alien Head Suckers
- Alioth (Devil Survivor 2)
- Alito
- All For One
- Allium Gyojan
- Allomon
- Alma Karma
- Alois Trancy
- Alpha Richter
- Alphamon
- Alucard (Hellsing)
- Alucard (Rosario+Vampire)
- Alus
- Aluze
- Alva (Pokémon)
- Amachi
- Amaimon
- Amata Kihara
- Amaterasu
- Amazon Quartet
- Amazon Trio
- Ameisha Kichougasaki
- Amelda
- Amemiya
- American Empire
- Amiba
- Amnael
- Amon (Devilman)
- Amon (Fist of the North Star)
- Amond
- Amshel Goldsmith
- Amy Kirio
- Anacondy
- Anastasia Romanova
- Anavel Gato
- Ancient Decepticons
- Ancient King
- AncientVolcanomon
- Andrea Cavalcanti
- Andreas
- Andrew Kersee Dunstan Francis Barbirolli
- Android 13
- Android 14
- Android 15
- Android 16
- Android 17
- Android 18
- Android 19
- Andromeda
- Andy Strauss
- Anemone
- Angel Dog/Devil Dog
- Angela Blanc
- Angelene
- Angelina Durless
- Angelus (Drakengard)
- Angila
- Angostura (Moomin)
- Anguished One
- Anige
- Animus (Fairy Tail)
- Anjuro "Angelo" Katagiri
- Anna (Freak Island)
- Anna Nishikinomiya
- Anna Williams
- Annie (Pokémon)
- Annie Leonhart
- Annin (Dragon Ball)
- Anthony Herzen
- Anti Spirit Team (Date A Live)
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