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He was voiced by Mark Hamill.
In "Memory Lane of Pain", The Powerpuff Girls remembered back to the time they fought with Popsicles. In the flashback, Popsicles was flying around on his ice cream sandwich saucer and laughing maniacally as he blasted people with his freezing lasers, turning them all into ice cream and popsicles.
The Powerpuff Girls came in to stop him and Popsicles blasted an ice laser at them to freeze them but they dodged it and he ended up turning the car behind them into an ice cream sundae. The Powerpuff Girls brainstormed a way to defeat him and Bubbles had the idea to blast him with a water hose to try and melt him. However, all she did was spray the hose all willy nilly and even squirting Blossom. Popsicles used the water to freeze Blossom and Bubbles into popsicles of themselves.
Buttercup went to save Blossom and Bubbles by using her frozen sisters as paddles to fight Popsicles and his popsicle swords in combat but Popsicles knocked Blossom out of her hands and smashed Bubbles to mush.
Buttercup got fed up with Popsicles and used her fire powers to melt him to death. After he melted, everything turned back to normal again and Buttercup got to keep one of his popsicle sticks as a souvenir.